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https://hdl.handle.net/2440/113573
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Type: | Journal article |
Title: | Hierarchical 1T-MoS₂ nanotubular structures for enhanced supercapacitive performance |
Other Titles: | Hierarchical 1T-MoS(2) nanotubular structures for enhanced supercapacitive performance |
Author: | Yang, S. Zhang, K. Wang, C. Zhang, Y. Chen, S. Wu, C. Vasileff, A. Qiao, S. Song, L. |
Citation: | Journal of Materials Chemistry A, 2017; 5(45):23704-23711 |
Publisher: | Royal Society of Chemistry |
Issue Date: | 2017 |
ISSN: | 2050-7488 2050-7496 |
Statement of Responsibility: | Shuang Yang, Ke Zhang, Changda Wang, Youkui Zhang, Shuangming Chen, Chuanqiang Wu, Anthony Vasileff, Shi-Zhang Qiao and Li Song |
Abstract: | Layered transition metal disulfides are currently being widely studied for advanced energy generation and storage applications. Here we report a facile template-assisted solvothermal strategy to obtain a hierarchical nanotubular structure consisting of ultrathin MoS₂ nanosheets with a metallic 1T phase. Synchrotron radiation based X-ray absorption fine structure (XAFS) and X-ray photoelectron spectroscopy (XPS) are used to investigate the structure and electronic properties of the 1T-MoS₂, which are largely different from annealed samples. Its hierarchical structure makes the obtained nanotubular 1T-MoS₂ an excellent electrode material for supercapacitors, with a high specific capacitance of 328.547 F g⁻¹ at a current density of 1 A g⁻¹ and 243.66 F g⁻¹ at a current density of 15 A g⁻¹. Moreover, the material displays excellent capacitance retention, retaining 98.4% capacity after 5000 cycles at a current density of 3 A g⁻¹. Notably, a high specific capacitance of 250 F g⁻¹ at 1 A g⁻¹ is also achieved in a two-electrode symmetrical cell, suggesting its great potential for new-generation supercapacitors. |
Rights: | This journal is © The Royal Society of Chemistry 2017 |
DOI: | 10.1039/c7ta08115d |
Published version: | http://dx.doi.org/10.1039/c7ta08115d |
Appears in Collections: | Aurora harvest 8 Chemical Engineering publications |
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