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https://hdl.handle.net/2440/114453
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dc.contributor.author | Azhar, M. | - |
dc.contributor.author | Abid, H. | - |
dc.contributor.author | Tade, M. | - |
dc.contributor.author | Periasamy, V. | - |
dc.contributor.author | Sun, H. | - |
dc.contributor.author | Wang, S. | - |
dc.date.issued | 2018 | - |
dc.identifier.citation | Chemical Engineering Journal, 2018; 341:262-271 | - |
dc.identifier.issn | 1385-8947 | - |
dc.identifier.issn | 1873-3212 | - |
dc.identifier.uri | http://hdl.handle.net/2440/114453 | - |
dc.description | Available online 08 February 2018 | - |
dc.description.abstract | In this paper, we demonstrate a cascade application of functional materials in adsorption and catalysis. Metal organic frameworks, MIL-96, were synthesized by a single solvent (water), and methanol (MIL-96-Me) or ethanol (MIL-96-Et) modulated method. Methanol modulation results in a change in porous structure and better CO2 adsorption and selectivity. After gas-phase adsorption of CO2, the MIL-96 can be reused for liquid-phase removal of water contaminants, demonstrating high capacities of para-hydroxybenzoic acid (p-HBA). Then, a transformation of the used MIL-96 by pyrolysis was employed to produce a metal oxide/C composite for catalytic activation of peroxymonosulfate (PMS) to degrade an organic pollutant, methyl orange. The composite exhibited excellent performance in the dye degradation. This study presents a proof of concept of integrated utilization of robust and functional nanomaterials for multiple applications without producing solid wastes after each use. | - |
dc.description.statementofresponsibility | Muhammad Rizwan Azhar, Hussein Rasool Abid, Moses O. Tade, Vijay Periasamy, Hongqi Sun, Shaobin Wang | - |
dc.language.iso | en | - |
dc.publisher | Elsevier BV | - |
dc.rights | © 2018 Elsevier B.V. All rights reserved. | - |
dc.source.uri | http://dx.doi.org/10.1016/j.cej.2018.02.030 | - |
dc.subject | MIL-96; CO₂adsorption; catalysis; personal care products; cascade application | - |
dc.title | Cascade applications of robust MIL-96 metal organic frameworks in environmental remediation: Proof of concept | - |
dc.type | Journal article | - |
dc.identifier.doi | 10.1016/j.cej.2018.02.030 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP150103026 | - |
dc.relation.grant | http://purl.org/au-research/grants/arc/DP170104264 | - |
pubs.publication-status | Published | - |
dc.identifier.orcid | Wang, S. [0000-0002-1751-9162] | - |
Appears in Collections: | Aurora harvest 3 Chemical Engineering publications |
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